This Hit and Run is a solid...as are the Part Deux.
What are your top 3 Room 101? I'll be honest I don't know one from the other.
Top three is tough. As I said earlier Lost and Found and Lost and Found Pard Deux are very enjoyable (although technically not Room 101 as they are a collaboration.
From Room 101, I really like all three of the Master Collection, Room 101 Connecticut, Namakubi which are all retired.
For those currently available, Farce (not Connecticut or Lonsdale) and The T (not the Connecticut versions) Breakfast in Portugal is my favorite of what I nicknamed the cartoon series (made for folks like CI)